Than the TePP and you will pentaphenylpyrrole (PPP), both TPM and you will TPM-Cl demonstrated extended emission frequencies. Due to its similar chemical substances structures, this is simply not plausible to trait the significant Stokes shift to help you variations in the energy gap between the low singlet thrilled county (S1) and you can ground state (S0). I therefore suggest that the brand new reddish emission corresponds to a minimal triplet happy condition (T1), that is lower than S1. 2, in which the contours are identical to their steady-county emission spectra, discussing the newest long lifetime features out of both TPM and you may TPM-Cl. The new lifetimes of one’s TPM and you may TPM-Cl crystalline powders is actually 20.step 1 and you can 8.9 μs, respectively (Fig. S3 and Dining table S1).

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Chongqing Wulong Karst Area, Wulong Karst Surroundings

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